ArticleChemistry (Weinheim an der Bergstrasse, Germany)2025
Engineering Alloxazines by Boron Coordination and Click Chemistry toward Small-molecule Fluorescent Probes.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Selective and strategic modification of redox cofactors offers significant advantages for the design of molecular probes, including high compatibility and affinity. This is particularly relevant in the case of redox cofactors with innate fluorescence properties, such as flavins, and synthetic strategies toward their functionalized analogues are of high interest to modulate properties. However, the synthetic elaboration of flavins and their alloxazine isomers still suffers from limitations. We report easy access to bioinspired fluorescent alloxazines with a boron difluorocatecholate moiety and explore the impact of core aromatic substitution on their photophysical properties. Further chemical elaboration through a CuAAC (copper-catalyzed azide-alkyne cycloaddition) click chemistry strategy opens the way to easy derivatization and further addressing.
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