Evidence map›Paper›PMID 40708318›Full record

ArticleAdvanced materials (Deerfield Beach, Fla.)2025

Nanometer Resolution Structure-Emission Correlation of Individual Quantum Emitters via Enhanced Cathodoluminescence in Twisted Hexagonal Boron Nitride.

Hanyu Hou, Muchuan Hua, Venkata Surya Chaitanya Kolluru, Wei-Ying Chen, Kaijun Yin, Pinak Tripathi, Maria K Y Chan, Benjamin T Diroll, Thomas E Gage, Jian-Min Zuo and 1 more

Abstract read
In one paragraph

Article in Advanced materials (Deerfield Beach, Fla.), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.

0numbers the graph read from it
0cells of the map it votes in
5citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

5 citing papers in PubMed.

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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

11 authors.

Hanyu HouCenter for Nanoscale Materials, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.
Muchuan HuaCenter for Nanoscale Materials, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.
Venkata Surya Chaitanya KolluruCenter for Nanoscale Materials, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.
Wei-Ying ChenNuclear Science and Engineering, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.
Kaijun YinDepartment of Materials Science and Engineering, Materials Research Laboratory, University of Illinois Urbana Champaign, 1304 W. Green St. MC 246, Urbana, IL, 61801, USA.
Pinak TripathiDepartment of Materials Science and Engineering, Materials Research Laboratory, University of Illinois Urbana Champaign, 1304 W. Green St. MC 246, Urbana, IL, 61801, USA.
Maria K Y ChanCenter for Nanoscale Materials, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.
Benjamin T DirollCenter for Nanoscale Materials, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.
Thomas E GageCenter for Nanoscale Materials, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.
Jian-Min ZuoDepartment of Materials Science and Engineering, Materials Research Laboratory, University of Illinois Urbana Champaign, 1304 W. Green St. MC 246, Urbana, IL, 61801, USA.
Jianguo WenCenter for Nanoscale Materials, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, IL, 60439, USA.ORCID https://orcid.org/0000-0002-3755-0044

Funding

Argonne National Laboratory, Laboratory Directed Research and Development DE-AC02-06CH11357Basic energy science Early Career award DE-AC02-06CH11357U.S. Department of Energy DE-AC02-06CH11357
6 · The paper itself

Abstract

Understanding the atomic structure of quantum emitters, often originating from point defects or impuritie, is essential for designing and optimizing materials for quantum technologies such as quantum computing, communication, and sensing. Despite the availability of atomic-resolution scanning transmission electron microscopy and nanoscale cathodoluminescence microscopy, experimentally determining the atomic structure of individual emitters is challenging due to the conflicting needs for thick samples to generate strong cathodoluminescence signals and thin samples for structural analysis. To overcome this challenge, significantly enhanced cathodoluminescence at twisted interfaces is leveraged to achieve sub-nanometer localization precision for the first time in mapping individual quantum emitters in carbon-implanted hexagonal boron nitride. This unprecedent spatial sensitivity, together with correlative electron energy loss spectroscopy quantitative scanning transmission electron microscopy imaging, and first principles density functional theory calculations, enables the identification of the atomic structure of the 440 nm blue emitter in hexagonal boron nitride as a substituted vertical carbon dimer. Building on the atomic structure insights, nanoscale spatially precise creation of blue emitters is demonstrated by electron beam irradiation of carbon-coated hexagonal boron nitride. This advancement in correlating atomic structures with optical properties lays the foundation for a deeper understanding and precise engineering of quantum emitters, significantly advancing the development of cutting-edge quantum information technologies.

Indexed as

2D materialatomic structurecathodoluminescencehexagonal boron nitridequantum emitterquantum information sciencesingle photon emittertwisted interface

Identifiers

PMID40708318
PMCPMC12531738

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.