ArticleIUCrJ2025
High-quality ultra-fast total scattering and pair distribution function data using an X-ray free-electron laser.
Article in IUCrJ, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Perspective: rethinking polymer crystallization pathways-two decades after Strobl's mesomorphic-to-granular-to-lamellar model.The European physical journal. E, Soft matter · 2026Article
- Structural evolution of iron oxides melts at Earth's outer-core pressures.Nature communications · 2026Article
- X-ray data reconstruction from incomplete data sampling.Journal of applied crystallography · 2025Article
- Atomistic Insights into Halide Double Perovskite Nanocrystals obtained by Multistep Synthesis and Efficient Compositional Engineering.ACS nano · 2025Article
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Authors and funding
51 authors.
Funding
Abstract
High-quality total scattering data, a key tool for understanding atomic-scale structure in disordered materials, require stable instrumentation and access to high momentum transfers. This is now routine at dedicated synchrotron instrumentation using high-energy X-ray beams, but it is very challenging to measure a total scattering dataset in less than a few microseconds. This limits their effectiveness for capturing structural changes that occur at the much faster timescales of atomic motion. Current X-ray free-electron lasers (XFELs) provide femtosecond-pulsed X-ray beams with maximum energies of ∼24 keV, giving the potential to measure total scattering and the attendant pair distribution functions (PDFs) on femtosecond timescales. We demonstrate that this potential has been realized using the HED scientific instrument at the European XFEL and present normalized total scattering data for 0.35 Å
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