Generative Artificial Intelligence for Synthetic Spectral Data Augmentation in Sensor-Based Plastic Recycling.

The reliance on deep learning models for sensor-based material classification amplifies the demand for labeled training data. However, acquiring large-scale, annotated spectral data for applications such as near-infrared (NIR) reflectance spectroscopy in plastic sorting remains a significant challenge due to high acquisition costs and environmental variability. This paper investigates the potential of large language models (LLMs) in synthetic spectral data generation. Specifically, it examines whether LLMs have acquired sufficient implicit knowledge to assist in generating spectral data and introduce meaningful variations that enhance model performance when used for data augmentation. Classification accuracy is reported exclusively as a proxy for structural plausibility of the augmented spectra; maximizing augmentation performance itself is not the study's goal. From as little as one empirical mean spectrum per class, LLM-guided simulation produced data that enabled up to 86% accuracy, evidence that the generated variation preserves class-distinguishing information. While the approach performs best for spectral distinct polymers, overlapping classes remain challenging. Additionally, the transfer of optimized augmentation parameters to unseen classes indicates potential for generalization across material types. While plastic sorting serves as a case study, the methodology may be applicable to other domains such as agriculture or food quality assessment, where spectral data are limited. The study outlines a novel path toward scalable, AI-supported data augmentation in spectroscopy-based classification systems.