ArticleThe journal of physical chemistry letters2025
Electron-Impact Resonances of Anthracene in the Presence of Methanol: Does the Solvent Identity Matter?
Article in The journal of physical chemistry letters, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Electron impact resonances of neutral molecules can be probed using 2D photoelectron spectroscopy of their radical anions, with a core advantage of being able to introduce solvent molecules in a systematic manner through clustering. This approach has been employed previously to probe the effect of water molecules on the resonances of anthracene. Here, we extend this study to probe the resonances of anthracene in the presence of methanol. We find that the nature of the solvent has little impact on the resonances from the perspective of the anion. Only the electron affinity is observed to increase, which corresponds to a concomitant decrease in resonance energy as viewed from a free electron impacting the anthracene-methanol cluster. For a critical cluster size,
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