ArticleActa crystallographica. Section A, Foundations and advances2025
Temporal ghost imaging for pump-probe X-ray solution scattering.
Article in Acta crystallographica. Section A, Foundations and advances, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Time-resolved small- and wide-angle X-ray scattering is a valuable tool for investigating biomolecular dynamics on a wide variety of timescales, without cryo-freezing or crystallization. However, some systems, such as the initial excitation of photo-active proteins, evolve dynamically on timescales that may be faster than the duration of the pump and probe beams. Data from a single pump-probe pulse pair therefore contain information from a mixture of time points. In this work, a simple algorithm is developed to recover the dynamics of solution scattering profiles. It leverages information about the pump and probe pulse beams' temporal profiles by using the same mathematical framework as ghost imaging [Pittman et al. (1995). Phys. Rev. A 52, R3429-R3432; Bennink et al. (2002). Phys. Rev. Lett. 89, 113601; Gatti et al. (2004). Phys. Rev. Lett. 93, 093602]. Results from several simulated data sets are presented.
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