ArticleNature communications2025
Simultaneous chirality and energy transfer of donor-acceptor chromophores via bio-inspired supramolecular light-harvesting.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Who cites it
2 citing papers in PubMed.
- Article
- Concurrent Generation of Tight and Loose Ion Pairs upon Charge-Transfer Excitation of Electron Donor-Acceptor Complexes in Solution.The journal of physical chemistry letters · 2026Article
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Authors and funding
6 authors.
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Abstract
The simultaneous transfer of chirality and energy is essential in biological systems, serving as a key inspiration for developing artificial analogs. Traditional methods, such as doping donor-acceptor chromophores into chiral gels or films, exhibit low chirality transfer efficiency due to inadequate stereo-communication. Here we present a bio-inspired strategy modeled on the chlorosomes of green bacteria. Specifically, platinated donor-acceptor chromophores form helical stacks, resembling the organization of bacteriochlorophylls in chlorosomes. Surfactant creates a confined hydrophobic environment, analogous to the role of glycolipids and phospholipids in chlorosomes, shielding the chromophores from water. This design enables energy and chirality transfer, as evidenced by femtosecond time-resolved circularly polarized luminescence spectroscopy. Further investigations reveal that amide units on the chromophores and stereochemical compatibility between donors and acceptors are critical for the dual information transfer. This study highlights the importance of a chlorosome-mimetic design in achieving simultaneous energy and chirality transfer in artificial systems.
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