ArticleApplied spectroscopy2026
Surface-Bulk Correlation Spectroscopy for the Characterization of Ternary Adsorption.
Article in Applied spectroscopy, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
A method is proposed whereby the range of equilibrium constants that describe how a ternary mixture of molecules is adsorbed onto a solid substrate may be obtained. This information may then be related to the surface preference of a particular species. The technique utilizes infrared and/or Raman spectra of the bulk phase, together with sum frequency generation spectra of the surface in a heterospectral two-dimensional correlation analysis. The method consists of a series of up to three experiments in which the bulk concentrations are varied, followed by a set of rules for interpreting the resulting correlation maps to identify adsorption sequences and surface preference. A scheme is provided to direct the design of the experiments and analyses for such multi-component mixtures.
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