ArticleProceedings of the National Academy of Sciences of the United States of America2025
Photothermal catalysis of waste plastics into propionic acid and hydrogen via Ni single-atom site isolation effect.
Shuai Yue, Yixiao Liu, Zhiyong Zhao, Guanshu Zhao, Mengxue Yang, Tao Zhang, Fei Li, Kewang Liu, Pengfei Wang, Sihui Zhan and 1 more
Abstract read
In one paragraphArticle in Proceedings of the National Academy of Sciences of the United States of America, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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5 · Who and what moneyAuthors and funding
11 authors.
Shuai Yue *Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.ORCID 0000-0001-7257-8539 Yixiao Liu *Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.
Zhiyong ZhaoMinistry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.ORCID 0009-0003-4207-0867 Guanshu ZhaoDepartment of Chemistry, University of Toronto, Toronto, ON M5S2E8, Canada.
Mengxue YangMinistry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.
Tao ZhangMinistry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.
Fei LiMinistry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.
Kewang LiuMinistry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.
Pengfei WangMinistry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.
Sihui ZhanMinistry of Education Key Laboratory of Pollution Processes and Environmental Criteria, College of Environmental Science and Engineering, Nankai University, Tianjin 300350, People's Republic of China.ORCID 0000-0002-1575-5946 Jinhu JiaChina Environment Publishing Group, Beijing 100062, People's Republic of China.
Funding
Frontiers Science Center for New Organic Matter 63181206Fundamental Research Funds for the Central Universities, Nankai University 63231195Fundamental Research Funds for the Central Universities, Nankai University 63253207MOST | National Natural Science Foundation of China (NSFC) 22076082MOST | National Natural Science Foundation of China (NSFC) 22225604 U24A20518Tianjin Commission of Science and Technology as key critical technologies R&D projects 23YFZCSN00010Young Scientific and Technologycal Talents (Level Two) in Tianjin QN20230206
6 · The paper itselfAbstract
Currently, catalytic recycling of polyethylene (PE) into high-value chemicals using solar energy often faces poor product selectivity and low efficiency. This is mainly due to the difficulty in effectively controlling the intermediates during PE photoreforming and the long-standing challenge of inefficient charge dynamics. Here, we present a solar-driven photothermal catalytic approach for the selective conversion of PE waste into propionic acid and hydrogen under ambient conditions. Atomically dispersed Ni sites supported on CeO
Indexed as
Ni single-atom sitesphotothermal catalysispolyethylene upcyclingpropionic acid productionsite isolation effect
Identifiers
PMID40569379
PMCPMC12232611
What OpenQuestion holds
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LicenceCC BY-NC-ND
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