ArticleNational science review2025
Integrated prelithiation and SEI engineering for high-performance silicon anodes in lithium-ion batteries.
Article in National science review, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Adsorption-Mediated Sodium Compensation for Hard Carbon Anodes Enabled by Soft-Contact Presodiation.Angewandte Chemie (International ed. in English) · 2026Article
- Facile Formation of Oxygen-Vacancy Gradient Enables In Situ Uniform Prelithiation in Vanadium Oxide Thin-Film Batteries.Angewandte Chemie (International ed. in English) · 2026Article
- Article
- Polymer-induced solid-electrolyte interphase on hard carbon enabling 5C fast-charging practical sodium-ion pouch cell.National science review · 2026Article
- Laser-Driven Single-Step Synthesis of Monolithic Prelithiated Silicon-Graphene Anodes for Ultrahigh-Performance Zero-Decay Lithium-Ion Batteries.Nano-micro letters · 2026Article
- Flame-retardant Cl-substituted electrolyte for low-temperature and high-voltage lithium-ion batteries with fast interfacial kinetics.National science review · 2026Article
- Beyond lithium-ion batteries: what's powering tomorrow's breakthroughs?National science review · 2025Article
Corrections and comments
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Authors and funding
11 authors.
Funding
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Abstract
Improving the initial Coulombic efficiency (ICE) of silicon anodes in lithium-ion batteries is a key challenge for enhancing their performance. Traditional prelithiation methods, such as using lithium naphthalenide (Li-Naph), are limited by the low lithiation potential of crystalline silicon, making them less effective for commercial applications. This study demonstrates that amorphous silicon anodes, with a higher lithiation potential, can be effectively prelithiated using Li-Naph. This prelithiation process also forms a robust solid electrolyte interphase, which significantly enhances the anode's cycling stability and overall battery performance. The prelithiated silicon anodes achieved a remarkable ICE improvement from 74.8% to 97.2% in full-cell tests. Furthermore, 27 mAh pouch cells exhibited excellent long-cycle stability and low-temperature performance, retaining 90.1% of their capacity after 800 cycles at 1 C. These findings highlight the potential for scalable prelithiation methods and open new avenues for advancing silicon anode technology in next-generation batteries.
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Registered trials
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