ArticleChemistry (Weinheim an der Bergstrasse, Germany)2025
Dynamics of Ligand and Guest in 1D Hg(II)-Bispidine Coordination Polymers With Different Topologies Investigated by Solid-State NMR.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
1D coordination polymers (CPs) made of parallel, weakly interacting chains have been recently proposed for the selective adsorption of volatile organic compounds (VOCs), one of the main sources of air and water pollution. Since the efficiency of adsorption for VOC removal strongly depends on the specific and stable interactions between the volatile species and the CP framework, the characterization at the atomic level of host-guest interactions and guest dynamics is of particular interest. Here, low- and high-resolution solid-state NMR experiments were applied to acquire information on ligand and guest dynamics for two 1D CPs (1-ClBz and 2-ClBz), both containing a bispidine organic ligand, Hg(II) as a metal center, and chlorobenzene trapped within the framework, but featuring different topologies. By combining analyses of on-resonance
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