ArticleScience advances2025
Liquid metal-induced low-temperature synthesis of tunable high-entropy oxides.
Article in Science advances, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Unlocking Low-Melting-Point and High-Conductivity Molten Salts via High-Entropy Strategy with Demonstration in Thermal Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- High-Temperature-Resistant Mid-Infrared Capability for Extreme Energy Systems.Nano-micro letters · 2026Review
- Self-adhesive high-entropy oxide sub-nanowire monolithic electrocatalysts.Nature nanotechnology · 2026Article
- Femtosecond laser synthesis of multiscale high-entropy alloys/graphene composites for high-performance Joule heating.Nature communications · 2026Article
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Authors and funding
2 authors.
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Abstract
High-entropy oxides (HEOs) have attracted attention due to their unique elemental synergistic effect and lattice distortion. However, mixing elements' vastly different radii and valences leads to substantial element segregation during the reaction. In addition, the requirement for a harsh temperature (1100°C) to achieve entropy stabilization results in the volatilization of low-melting point components. Here, we propose a strategy for synthesizing functionalized Ga-based HEOs (GHEOs) at a low temperature (400°C) by the Ga integration mechanism. The negative mixing enthalpy between Ga and other metals reduces the Gibbs free energy, enabling the creation of homogeneous GHEOs through a hydrothermal process at a lower temperature. The Ga integration mechanism is supported by thermodynamic and density functional theory analyses. In particular, the perovskite, spinel, and rock salt crystal can be precisely tuned by choosing metal ions, enabling tailored applications in electrocatalysis, energy-saving materials, and methane sensors. Hence, this GHEOs strategy can be extended to realize many ideal GHEOs adjusted for specific applications.
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Registered trials
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