ArticleChemistry (Weinheim an der Bergstrasse, Germany)2025
Aggregation, Photoluminescence, and Cytotoxicity of Pt(II) and Re(I) Complexes Bearing Multimodal-Coordinating Luminophores.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
In this study, a polydentate ligand capable of adopting multiple coordination modes (N*N, C^N*N, and C^N*N^C) was established. Depending on the chelation conditions and the co-ligand used in the subsequent steps, nine complexes became accessible. The four Pt(II)-based species with N*N-coordination motif show tunable emission and cytotoxicity. Two Pt(II) complexes with C^N*N-type coordination were also obtained, and the exchange of the co-ligand from chlorido to cyanido led to an enhancement in the photoluminescence quantum yield from <0.02 to 0.55. These compounds exhibit distinct solid-state characteristics associated with Pt⋯Pt-interactions. Interestingly, the tetradentate C^N*N^C-coordination mode was not accessible, most likely due to kinetic reasons and insolubility-related purification hurdles. However, the use of a N*N-coordination mode for a Re(I) center yielded non-cytotoxic
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