ArticleNature communications2025
Electronic strong coupling modifies the ground-state intermolecular interactions in self-assembled chlorin molecules.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
What it found
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Who cites it
6 citing papers in PubMed.
- Emissive BN-Embedded Cumulenes: Synthesis and Bidirectional Photocurrent Modulation.Angewandte Chemie (International ed. in English) · 2026Article
- Direct Readout of Excited-State Lifetimes in Chlorin Chromophores under Electronic Strong Coupling.Journal of the American Chemical Society · 2026Article
- Collectively-Modified Intermolecular Electron Correlations: The Connection of Polaritonic Chemistry and Spin Glass Physics.Chemical reviews · 2026Review
- Density-functional tight binding meets Maxwell: unraveling the mysteries of (strong) light-matter coupling efficiently.Nanophotonics (Berlin, Germany) · 2025Article
- Toward Polaritonic Molecular Orbitals for Large Molecular Systems.Journal of chemical theory and computation · 2024Article
- Analytical Evaluation of Ground State Gradients in Quantum Electrodynamics Coupled Cluster Theory.Journal of chemical theory and computation · 2024Article
Corrections and comments
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Authors and funding
6 authors.
Funding
Abstract
The strong coupling of a molecular electronic transition with a quantized radiation field can result in modified photophysics compared to its uncoupled counterparts. Often, such changes are attributed to kinetic factors, overlooking the possible modifications to intermolecular interactions. The spin-cast films of chlorin e6 trimethyl ester (Ce6T) show an excitonic coupling band in absorption resulting from their ground-state intermolecular interactions and subsequent excimer-like emission upon photoexcitation. Interestingly, the electronic strong coupling (ESC) of the Ce6T Soret and Q-band suppresses the intermolecular excitonic interactions that otherwise exist in the Ce6T thin films and brings back the monomer-like emission characteristics. Our experiment provides a unique tool to tune the molecular assembly without involving chemical modifications. Our results suggest that ESC can induce modification to the intermolecular interaction forces that hold together the molecular assemblies in the ground state, which is a significant step toward understanding the fundamentals of polaritonic chemistry in detail.
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Registered trials
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