ArticleJournal of solid state electrochemistry : current research and development in science and technology2025
Are redox catalytic reaction rates accelerated in microdroplets on electrode surfaces?
Article in Journal of solid state electrochemistry : current research and development in science and technology, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Homogeneous redox catalysis within electrochemically supported microdroplets immobilised on an electrode surface and bathed by an immiscible electrolyte solution is characterised using finite difference numerical methods, after conformal transformation of the physical problem. This is shown to be a challenging environment to simulate and model, not least due to the confinement of the heterogeneous electron transfer to the droplet/support/electrolyte boundary, and hence leading to acute convergent/divergent diffusion regimes. Reactivity at the triple phase boundary underpins both the spatial and temporal non-uniformity of the reacting droplet environment. Crucially, through comparison with experimental data reported in the literature, it is demonstrated that Supplementary Information: The online version contains supplementary material available at 10.1007/s10008-025-06283-4.
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