ArticleJournal of the American Chemical Society2025
Closed-Loop Framework for Discovering Stable and Low-Cost Bifunctional Metal Oxide Catalysts for Efficient Electrocatalytic Water Splitting in Acid.
Article in Journal of the American Chemical Society, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Pre-catalysts for the hydrogen evolution reaction: from dynamic reconstruction to rational design.Chemical science · 2026Review
- Materials Databases: Foundations of Modern Digital Materials.Precision chemistry · 2026Review
- Accelerated discovery of highly stable ruthenium-based high-entropy oxides for acidic oxygen evolution.Science advances · 2026Article
- Digital materials ecosystem: from databases to AI agents for autonomous discovery.Chemical science · 2026Review
- Decoding heterogeneous electrocatalysts for acidic oxygen evolution: mechanisms, rational design and AI acceleration.National science review · 2025Review
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Authors and funding
12 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Electrocatalytic water splitting, comprising the oxygen evolution reaction (OER) and hydrogen evolution reaction (HER), provides a sustainable route for hydrogen production. While low-cost metal oxides (MOs) are appealing as alternatives to noble metal electrocatalysts, their application in acidic media remains challenging. However, the dynamic nature of some MO surface structures under electrochemical conditions offers an opportunity for rational catalyst design to achieve bifunctionality in acidic OER and HER. Here, we present a closed-loop framework that integrates potential catalyst exploration (front-end), synthesis and electrochemical tests (mid-end), and advanced characterizations (back-end). This framework combines crucial steps in electrocatalyst exploration, including data mining, surface state analysis, microkinetic modeling, and proof-of-concept experiments to identify stable and cost-effective MO catalysts for acidic water splitting. Using this approach, RbSbWO
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