ArticleNature communications2025
Co-initiating-system dual-mechanism drives the design of printable entangled polymer multinetworks.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
What it found
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Who cites it
5 citing papers in PubMed.
- Chain entanglement-stabilized injectable zwitterionic hydrogel for vitreous replacement and retinal tamponade.National science review · 2026Article
- Resolving the Strength-Modulus-Elasticity Tradeoff in Elastomers Using Dual Phase-Separated Nanodomains.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Rapid photocontrollable dopamine polymerization for instant adaptive wet adhesion.Nature communications · 2026Article
- Dual-Terminal Molecular Strategy for Robust and Reversible Supramolecular Adhesion.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Fully Aqueous and Printable Photonic Inks with Tunable Pitch and Optical Memory via Hydrogen-Bonded HPC-PVA Networks.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
Corrections and comments
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Authors and funding
8 authors.
Funding
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Abstract
Entanglement significantly enhances the mechanical performance and functionality of both natural and synthetic materials. However, developing straightforward, versatile strategies for creating high-performance entangled polymer materials remains a challenge. Here, a co-initiating-system dual-mechanism strategy is designed for fabricating printable entangled polymer multinetworks. This thermal-light dual-initiation process benefits the synthesis of high-molecular-weight polymers and promotes the rapid formation of multinetworks within hydrogels. The resulting long polymer chains enable hydrogels with higher mechanical performance, lower stress relaxation, and activation energy compared to short polymer chain-contained samples. Such a method proves more effective than traditional self-thickening and strengthening techniques for enhancing hydrogel entanglements and is also compatible with additive manufacturing, enabling the design of complex 2D webs with adaptive mechanical performance and capable of detecting and sensing applications. This work provides an effective strategy for designing high-performance entangled polymer materials, which are set to impact numerous fields, from advanced sensing to material science and beyond.
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Registered trials
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