ArticleNature communications2025
Unlocking single-atom induced electronic metal-support interactions in electrocatalytic one-electron water oxidation for wastewater purification.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
What it found
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The trial behind it
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Who cites it
10 citing papers in PubMed.
- Electron-Rich Nickel Enabled by Charge Transfer in Multimetal Nanostructures for Efficient Ammonia-to-Hydrogen Conversion.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Self-reconstruction of single copper atoms drives precise hydroxyl radicals generation for efficient water disinfection.Nature communications · 2026Article
- Interfacial Acid Sites-Mediated ZnO-Based Electrocatalysts for Sustainable Dual-Pathway HAdvanced materials (Deerfield Beach, Fla.) · 2026Article
- Beyond the Active Site: Hydrophobic Microenvironment Engineering for Single-Atom Catalysts.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Programming Insulator-to-Metallic Transport in Insulating Materials via Surface Single-Atom Engineering.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Industrial electrocatalytic C-C coupling reaction of CNational science review · 2026Article
- Electronic structure manipulation in electrocatalysis: mechanisms and design principles.Chemical science · 2026Review
- Selective Biomass Valorization via Cascade Photooxidation and Photothermal Hydride Shift.Journal of the American Chemical Society · 2026Article
- Integrating Overall Water Splitting with Advanced Oxidation for Wastewater Treatment Using a Bifunctional Medium-Entropy Amorphous Alloy.Nano-micro letters · 2026Article
- Decoding the Stability-Activity Paradox in Electrochemical Ammonia Oxidation: An Operando Perspective.ACS omega · 2026Review
Corrections and comments
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Authors and funding
4 authors.
Funding
Abstract
Electro-oxidation is a promising green technology for decentralized wastewater purification. However, its efficacy is primarily constrained by the selectivity and efficiency of hydroxyl radical (•OH) generation through one-electron water oxidation. In this study, we elucidate the mechanism of electronic metal-support interactions (EMSI) of Ni single-atoms on antimony-doped tin oxide anode (Ni/ATO) to enhance •OH production and overall water treatment efficiency. We experimentally and theoretically investigate both the structural evolution process and micro-interface mechanisms associated with the EMSI effects induced by Ni single-atoms. The optimized electronic structures in the interfacial catalysts under EMSI conditions and the co-catalytic role of Ni single-atoms synergistically facilitate selective and efficient •OH generation, resulting in over a fivefold increase in its steady-state concentration and tenfold enhancement in pseudo-first-order rate constant of sulfamethoxazole degradation compared to those on bare ATO. With the EMSI, rapid electron transfer channels were established for a marked enhancement in the adsorption, conversion, and dissociation of interfacial H
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Registered trials
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