ArticleACS applied materials & interfaces2025
Ionic Associations and Hydration in the Electrical Double Layer of Water-in-Salt Electrolytes.
Article in ACS applied materials & interfaces, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Thermodynamic effects of solid electrolyte interphase formation from solvation and ionic association in water-in-salt electrolytes.Faraday discussions · 2026Article
- Nonmonotonic Screening and Solvation Dynamics of the Electrical Double Layer in Concentrated Lithium Salt Electrolytes.Nature communications · 2026Article
- Reversible ionic aggregation kinetics in concentrated electrolytes.Chemical science · 2026Article
- Water doping sodium battery electrolyte controls nanostructure, interactions, and electrochemical properties.Science advances · 2026Article
- Theory of Cation Solvation in the Helmholtz Layer of Li-Ion Battery Electrolytes.ACS applied energy materials · 2025Article
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Authors and funding
6 authors.
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Abstract
Water-in-Salt-Electrolytes (WiSEs) are an exciting class of concentrated electrolytes finding applications in energy storage devices because of their expanded electrochemical stability window, good conductivity and cation transference number, and fire-extinguishing properties. These distinct properties are thought to originate from the presence of an anion-dominated ionic network and interpenetrating water channels for cation transport, which indicates that associations in WiSEs are crucial to understanding their properties. Currently, associations have mainly been investigated in the bulk, while little attention has been given to the electrolyte structure near electrified interfaces. Here, we develop a theory for the electrical double layer (EDL) of WiSEs, where we consistently account for the thermoreversible associations of species into Cayley tree aggregates. The theory predicts an asymmetric structure of the EDL. At negative voltages, hydrated Li
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