ArticleAdvanced materials (Deerfield Beach, Fla.)2025
In Situ Polymerized Polyfluorinated Crosslinked Polyether Electrolytes for High-Voltage Lithium Metal Batteries.
Article in Advanced materials (Deerfield Beach, Fla.), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Zwitterionic Dynamic Supramolecular Elastomer Electrolytes for High-Voltage and Dendrite-Free Lithium Metal Batteries.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- A Rigid-Flexible Polyinterface Enabling Molecular-Level Dual-Ion Regulation for Ultrastable Lithium Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- High energy density quasi-solid-state lithium batteries usingChemical science · 2026Review
- Polyrotaxane-Assembled Semi-Interpenetrating Polymer Electrolytes Enabling High-Voltage Lithium Metal Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- In situ anchoring 2D hexagonal Zn-MOF on MXene toward robust anode-less 5 V-class Li metal batteries.Science advances · 2026Article
- Uniform and High LiSmall (Weinheim an der Bergstrasse, Germany) · 2025Review
- Molecular Design of Difluorinated Polyether Electrolyte for Ultrastable High-Voltage All-Solid-State Lithium Metal Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- In Situ Polymerized Polyfluorinated Crosslinked Polyether Electrolytes for High-Voltage Lithium Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2025Article
Corrections and comments
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Authors and funding
10 authors.
Funding
Abstract
In situ polymerized polyether electrolytes are promising for solid-state Li metal batteries due to their high ionic conductivity and excellent interfacial contact. However, their practical application is hindered by Li dendrite formation, interfacial degradation, and limited oxidative stability. Herein, we propose an in situ polymerized polyfluorinated crosslinked polyether electrolyte (PDOL-OFHDBO), synthesized by copolymerizing 1,3-dioxolane (DOL) with 2,2'-(2,2,3,3,4,4,5,5-octafluorohexane-1,6-diyl)bis(oxirane) (OFHDBO) as a polyfluorinated crosslinker. The electron-withdrawing polyfluorinated groups endow PDOL-OFHDBO with enhanced oxidative stability and interfacial compatibility, while reducing the solvation power of the polymer matrix to promote an anion-derived inorganic-rich solid electrolyte interphase for uniform Li deposition. Consequently, PDOL-OFHDBO exhibits a wide electrochemical stability window (>5.6 V) and enables long-term stable Li plating/stripping for over 1100 h. Furthermore, Li||LiNi
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