Evidence map›Paper›PMID 40312520›Full record

ArticleNature communications2025

Unveiling a large fraction of hidden organosulfates in ambient organic aerosol.

Jialiang Ma, Natalie Reininger, Cunliang Zhao, Damian Döbler, Julian Rüdiger, Yanting Qiu, Florian Ungeheuer, Mario Simon, Luca D'Angelo, Anna Breuninger and 12 more

Abstract read
In one paragraph

Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

22 authors.

Jialiang MaInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany. ma@iau.uni-frankfurt.de.ORCID http://orcid.org/0000-0003-0815-4066
Natalie ReiningerInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany.ORCID http://orcid.org/0000-0002-5018-2901
Cunliang ZhaoSchool of Earth Science and Engineering, Hebei University of Engineering, Handan, China.
Damian DöblerAir Monitoring Network, German Environment Agency, Langen, Germany.
Julian RüdigerAir Monitoring Network, German Environment Agency, Langen, Germany.
Yanting QiuState Key Joint Laboratory of Environmental Simulation and Pollution Control, Peking University, Beijing, China.ORCID http://orcid.org/0000-0003-2632-8621
Florian UngeheuerInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany.ORCID http://orcid.org/0000-0002-4557-3844
Mario SimonInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany.
Luca D'AngeloInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany.ORCID http://orcid.org/0000-0002-5518-2361
Anna BreuningerInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany.ORCID http://orcid.org/0009-0009-6684-0380
Julia DavidInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany.ORCID http://orcid.org/0009-0000-9913-0611
Yanxin BaiCollege of Environmental Science and Engineering, Hunan University, Changsha, China.
Yushan LiCollege of Environmental Science and Engineering, Hunan University, Changsha, China.
Ying XueCollege of Environmental Science and Engineering, Hunan University, Changsha, China.
Lili LiCollege of Environmental Science and Engineering, Hunan University, Changsha, China.
Yuchen WangCollege of Environmental Science and Engineering, Hunan University, Changsha, China.
Stefanie HildmannInstitute of Inorganic and Analytical Chemistry, Johannes Gutenberg-University, Mainz, Germany.ORCID http://orcid.org/0000-0002-9844-9556
Thorsten HoffmannInstitute of Inorganic and Analytical Chemistry, Johannes Gutenberg-University, Mainz, Germany.
Bangjun LiuSchool of Earth Science and Engineering, Hebei University of Engineering, Handan, China.
Hongya NiuSchool of Earth Science and Engineering, Hebei University of Engineering, Handan, China.
Zhijun WuState Key Joint Laboratory of Environmental Simulation and Pollution Control, Peking University, Beijing, China.
Alexander L VogelInstitute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany. vogel@iau.uni-frankfurt.de.ORCID http://orcid.org/0000-0002-1293-6370

Funding

Deutsche Forschungsgemeinschaft (German Research Foundation) 428312742
6 · The paper itself

Abstract

Organosulfates are key compounds driving the anthropogenic enhancement of ambient organic aerosol, however, total organosulfate quantification remains elusive due to their molecular diversity and the scarcity of authentic standards. Here, we present a solid-phase extraction method that isolates organosulfates from ambient aerosol samples and enables their identification and quantification using mass spectrometry and a charged aerosol detector, respectively. We investigate ambient aerosol samples from urban China and rural Germany and quantify ~130 and ~65 chromatographically resolved organosulfates, respectively, contributing less than ~2% to the total organic matter. We find a significantly larger organosulfate fraction appearing as a broad peak in the chromatograms from the charged aerosol detector. Confirming its origin from chromatographically non-resolved organosulfates, an all-ion fragmentation experiment reveals specific sulfate-related ions. Integrating this peak, we find the contribution of organosulfates to organic aerosol is 12-17% and ~21% in samples from urban China and rural Germany, respectively. These findings emphasise the potential of sulfur emission reduction for mitigating both sulfate-related and organic aerosol pollution.

Identifiers

PMID40312520
PMCPMC12046013

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.