ArticleACS applied polymer materials2025
Structure-Property Behavior of Hydroxyl-Terminated Polybutadiene-Based Urethanes Additionally Cross-Linked Using Sustainable Biosourced Rosin Esters.
Article in ACS applied polymer materials, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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8 authors.
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Abstract
Hydroxyl-terminated polybutadiene (HTPB) particularly when cross-linked with a diisocyanate is a very versatile elastomer having excellent mechanical and low temperature properties suitable for applications as diverse as binders in rocket propellants to surface coatings. These properties can be tailored further by the inclusion of a plasticizer, e.g., octadecyl adipate, but there are many technical challenges remaining around the use of such plasticizers, including migration from and miscibility with HTPB, together with the problem that such plasticizers are synthesized from non-renewable feedstocks. To address these limitations, rosin and functional rosin esters, sourced from pine trees, were blended with HTPB at loadings up to 20 wt % prior to cross-linking with toluene diisocyanate. All rosin esters studied were shown to be fully miscible with HTPB; a single glass transition temperature (
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