ArticleChemSusChem2025
Multiplexed and Membraneless Redox-Mediated Electrochemical Separations Through Bipolar Electrochemistry.
Article in ChemSusChem, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Authors and funding
3 authors.
Funding
Abstract
Redox-active electrosorbents are promising platforms for selective separations. However, these platforms face intrinsic challenges in extracting multiple species simultaneously, as their binding mechanisms are typically tailored to separate a single ion preferentially. Here, bipolar electrochemistry is leveraged to introduce a new strategy for the multiplexed use of redox-active and capacitive materials for separations. Using polyvinyl ferrocene (PVF)-, Prussian blue analog (PBA)-functionalized, and carbon-based electrodes, multicomponent separations within a modular bipolar electrode (BPE) platform are demonstrated. The multiplexed BPE system provides distinct electrochemical environments within each BPE pair, enabling parallel selective separations. With three identical PVF BPEs, arsenic uptake increased linearly from 41.4 to 115.4 mg
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