ArticleChemical science2025
Tailored engineering of primary catalytic sites and secondary coordination spheres in metalloenzyme-mimetic MOF catalysts for boosting efficient CO
Jiawei Li, Fan Yang, Benling Yu, Zhongke Dai, Shiyuan Wei, Ying Wu, Liuqing He, Fa Zhou, Jianhan Huang, You-Nian Liu
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In one paragraphArticle in Chemical science, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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10 authors.
Jiawei LiCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.ORCID https://orcid.org/0000-0001-5646-198X Fan YangCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.
Benling YuCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.
Zhongke DaiCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.
Shiyuan WeiCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.
Ying WuGuangDong Engineering Technology Research Center of Modern Fine Chemical Engineering, School of Chemical Engineering and Light Industry, Guangdong University of Technology Guangzhou 510006 P. R. China.
Liuqing HeThe Second Xiangya Hospital of Central South University Changsha 410000 Hunan P. R. China.
Fa ZhouCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.
Jianhan HuangCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.ORCID https://orcid.org/0000-0002-3838-0622 You-Nian LiuCollege of Chemistry and Chemical Engineering, Hunan Provincial Key Laboratory of Micro and Nano Material Interface Science, Central South University Changsha 410083 Hunan P. R. China lijiawei@csu.edu.cn jianhanhuang@csu.edu.cn.ORCID https://orcid.org/0000-0002-7078-5937 Funding
No grant is acknowledged in the PubMed record.
6 · The paper itselfAbstract
The fabrication of metalloenzyme-mimetic artificial catalyst is a promising approach to achieve maximum catalytic efficiency, but the rational integration of sophisticatedly optimized primary catalytic sites (PCS) and secondary coordination spheres (SCS) for specific transformation poses a grand challenge. Here in this work, we report the tailored engineering of Cu PCS and perfluoroalkyl SCS onto a zirconium-based framework [UiO-67-(BPY-Cu)-F
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PMID40248246
PMCPMC12000916
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