Probing the Limits of Mechanical Stability of the Mesoporous Metal-Organic Framework DUT-76(Cu) by Hydrocarbon Physisorption.

Kai Konowski, Volodymyr Bon, Martin A Karlsen, Martin Etter, Nadine Bönisch, Ankita De, Stefan Kaskel

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Article in ACS applied materials & interfaces, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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7 authors.

Kai KonowskiChair of Inorganic Chemistry I, Technische Universität Dresden, Bergstraße 66, Dresden 01069, Germany.

Volodymyr BonChair of Inorganic Chemistry I, Technische Universität Dresden, Bergstraße 66, Dresden 01069, Germany.ORCID 0000-0002-9851-5031

Martin A KarlsenP02.1 Beamline, PETRA III Synchrotron, DESY, Notkestraße 85, Hamburg 22607, Germany.ORCID 0000-0003-1262-8965

Martin EtterP02.1 Beamline, PETRA III Synchrotron, DESY, Notkestraße 85, Hamburg 22607, Germany.

Nadine BönischChair of Inorganic Chemistry I, Technische Universität Dresden, Bergstraße 66, Dresden 01069, Germany.

Ankita DeChair of Inorganic Chemistry I, Technische Universität Dresden, Bergstraße 66, Dresden 01069, Germany.ORCID 0000-0003-4962-0510

Stefan KaskelChair of Inorganic Chemistry I, Technische Universität Dresden, Bergstraße 66, Dresden 01069, Germany.ORCID 0000-0003-4572-0303

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6 · The paper itself

Abstract

The mechanical robustness of MOFs is crucial in most adsorption-related applications. Herein, we investigated the interaction of the mesoporous metal-organic framework DUT-76(Cu) with various C1-C4 hydrocarbons at their boiling points. During adsorption, the pore structure partially collapsed into an amorphous phase while retaining a residual porosity. We employed a combination of multicycle physisorption experiments using different hydrocarbons (methane, ethane, ethylene, propane, propylene,

Indexed as

adsorption, DUT-76, total scattering, n-alkanes, n-alkenes, crystal size, metal−organic frameworks

Identifiers

PMID40196993

DOI10.1021/acsami.5c00164

PMCPMC12022944

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