ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2025
Fluorinated Alkyl Chains Terminated Polar Glycol Ether Side Chain for N-Type Organic Thermoelectrics with Enhanced Performance and Air Stability.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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3 citing papers in PubMed.
- New-Era Polymer Thermoelectrics: Material Innovations, Doping Frontiers, Decoupling Strategies, and Unconventional Applications.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- High-gain and broadband in vivo amplifiers enabled by matched materials.Nature communications · 2026Article
- Fluorinated Alkyl Chains Terminated Polar Glycol Ether Side Chain for N-Type Organic Thermoelectrics with Enhanced Performance and Air Stability.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
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5 authors.
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Abstract
N-type organic thermoelectric materials with excellent device performance and air stability are critically important for practical applications in organic thermoelectric devices. However, the design and synthesis of air-stable n-type conductive materials with high electrical conductivities remain a significant challenge. In this paper, a new strategy is reported to enhance the thermoelectric performance and air stability of naphthalenediimide (NDI)-dialkoxybithiazole-based conjugated polymers by introducing fluorinated alkyl chains terminated polar glycol ether side chains into the NDI unit. After molecular doping with 4-(2,3-dihydro-1,3-dimethyl-1H-benzoimidazol-2-yl) phenyl)-N, N-dimethylbenzenamine (N-DMBI), the doped films of the fluorinated alkyl side-chain modified conjugated polymer exhibit higher electrical conductivity, thus resulting in a greater power factor; and better air stability compared to those of the unmodified polymer with the same conjugated backbone. The work provides insights into material design for the future development of air-stable n-type organic thermoelectrics.
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