ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2025
Surface Engineering-Induced d-Band Center Down-Regulation in High-Entropy Alloy Nanowires for Enhanced Nanozyme Catalysis.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
What it found
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Who cites it
6 citing papers in PubMed.
- High Entropy Effect Induced In-situ Surface Hydroxylation for Robust Electro-assisted Uranium Mineralization from Real Nuclear Wastewater.Nature communications · 2026Article
- Deciphering the Catalytic Mechanism of Oxidoreductase-Like Nanozymes Along the Reaction Pathway: Activity, Specificity and Sustainability.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Spatially confined multi-enzyme cascade nanoreactor for portable and real-time pesticide detection.Journal of nanobiotechnology · 2026Article
- Colorimetric detection of amino acids enabled by functional nanomaterials: mechanisms, performance evaluation, and translational perspectives.Mikrochimica acta · 2026Review
- High-entropy alloy Janus artificial enzymes for pH-gated sequential redox therapy of drug-resistant bacterial infection.Nature communications · 2026Article
- Surface Engineering-Induced d-Band Center Down-Regulation in High-Entropy Alloy Nanowires for Enhanced Nanozyme Catalysis.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
Corrections and comments
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Authors and funding
11 authors.
Funding
Abstract
High-entropy alloys (HEAs) have garnered extensive attention owing to their broad compositional tunability and high catalytic activity. However, precisely modulating the enzyme-like activity of HEAs and enhancing their biocompatibility for biological applications remain severely challenging. Herein, PtRuFeCoNi HEA nanowires (NWs) are synthesized by adjusting the metal composition and surface-engineered with polydopamine (PDA) to form HEA NWs@PDA nanozymes (HEzymes@PDA) with superior catalytic activity and photothermal properties. Density functional theory calculations and the Sabatier principle reveal that self-polymerized PDA surface engineering moderately lowers the d-band center of the HEAs, optimizes the surface charge distribution, and enhances the adsorption-desorption efficiency of the substrates. As a proof-of-concept, the HEzymes@PDA are synergistically integrated with hydrogels for biosensing analysis. This study presents an innovative paradigm for designing highly active HEA nanozymes via surface engineering and demonstrates their immense potential in catalytic sensing applications.
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Registered trials
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