ArticleJournal of the American Chemical Society2025
Impact of Noncompensating Ions on the Electrochemical Performance of n-Type Polymeric Mixed Conductors.
Article in Journal of the American Chemical Society, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
3 citing papers in PubMed.
- Structure-Driven Ion Transport in Conjugated Polymers with Crown Ether Side Chains: From the Nano- to Microscale.Chemistry of materials : a publication of the American Chemical Society · 2026Article
- Doping-Free Polymer Nanoparticle Engineering of n-Type Organic Mixed Ion-Electron Conductors for Enhancement-Mode Organic Electrochemical Transistors.Macromolecular rapid communications · 2026Article
- High-Performance Ambipolar Organic Electrochemical Transistors Based on Diketopyrrolopyrrole-Dialkoxybithiazole Conjugated Polymers for Single-component Inverters.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
Corrections and comments
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Authors and funding
11 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Organic mixed ionic-electronic conductors (OMIECs) have emerged as essential materials for applications in bioelectronics, neuromorphics, and energy storage, owing to their ability to transport both ions and electrons. While significant progress has been made in understanding their operation, the role of noncompensating ions in polymer redox processes remains underexplored, particularly in the context of their impact on charge compensation and device performance. In this study, we systematically investigate the influence of noncompensating ions on the performance of n-type OMIECs with and without polar side chains, focusing on their interactions with electrolytes containing anions from the Hofmeister series. Our findings reveal a stark contrast in charging behavior and organic electrochemical transistor (OECT) performance based on side-chain chemistry. Polar oligoether side chains promote interactions with anions, resulting in significant performance variations. We demonstrate the critical role of polymer side-chain interactions with the different anions, where polyatomic anions capable of infiltrating the film degrade device performance, particularly in terms of transconductance and operational stability. In contrast, OMIECs without side chains exhibit performance independent of the noncompensating ion nature. Through electrochemical analysis, spectroscopic techniques, and molecular dynamics simulations, we provide a comprehensive understanding of how ion incorporation and polymer-electrolyte interactions shape device behavior. This study highlights the transformative role of side-chain functionality in tailoring the properties of the OMIEC and offers a design framework for high-performance OECTs, enabling advancements in biosensing, neuromorphic computing, and beyond.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.