ArticleThe journal of physical chemistry. B2025
Exceptionally Strong Double-Layer Barriers Generated by Polyampholyte Salt.
Article in The journal of physical chemistry. B, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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1 citing paper in PubMed.
- Classical Density Functional Treatment of Polydisperse Polarizable Clusters.The journal of physical chemistry. B · 2026Article
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3 authors.
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Abstract
Experiments using the surface force apparatus have found anomalously long-range interactions between charged surfaces in concentrated salt solutions. Ion clustering has been suggested as a possible origin of this behavior. In this work, we demonstrate that if such stable clusters indeed form, they are able to induce remarkably strong free energy barriers under conditions where a corresponding solution of simple salt provides negligible forces. Our cluster model is based on connected ions producing a polyampholyte salt containing a symmetric mixture of monovalent cationic and anionic polyampholytes. Ion distributions and surface interactions are evaluated utilizing statistical-mechanical (
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