Evidence map›Paper›PMID 40172133›Full record

ArticleEnvironmental science & technology2025

Spatiotemporal Trend of PFAS in Estuarine Sediments: Insights into Chlorinated Polyfluoroalkyl Ether Sulfonate Transformation.

Qi Wang, Yuefei Ruan, Yetong Shao, Linjie Jin, Naiyu Xie, Xiaoqiang Yang, Yuanyuan Hong, He Wang, Akira Tsujimoto, Moriaki Yasuhara and 2 more

Abstract read
In one paragraph

Article in Environmental science & technology, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

12 authors.

Qi WangState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.ORCID 0000-0002-3156-9246
Yuefei RuanState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.ORCID 0000-0003-4696-5708
Yetong ShaoState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.
Linjie JinState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.
Naiyu XieState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.
Xiaoqiang YangSouthern Marine Science and Engineering Guangdong Laboratory (Zhuhai), Zhuhai 519080, China.
Yuanyuan HongSchool of Biological Sciences, Area of Ecology and Biodiversity, Swire Institute of Marine Science, Institute for Climate and Carbon Neutrality, and Musketeers Foundation Institute of Data Science, The University of Hong Kong, Hong Kong SAR 999077, China.
He WangSchool of Biological Sciences, Area of Ecology and Biodiversity, Swire Institute of Marine Science, Institute for Climate and Carbon Neutrality, and Musketeers Foundation Institute of Data Science, The University of Hong Kong, Hong Kong SAR 999077, China.
Akira TsujimotoInstitute of Education, Academic Assembly, Shimane University, Matsue, Shimane 690-8504, Japan.
Moriaki YasuharaState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.
Kenneth Mei Yee LeungState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.ORCID 0000-0002-2164-4281
Paul K S LamState Key Laboratory of Marine Pollution (SKLMP), City University of Hong Kong, Hong Kong SAR 999077, China.ORCID 0000-0002-2134-3710

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Per- and polyfluoroalkyl substances (PFAS) are synthetic long-lasting chemicals. Marine sediment is a major repository for PFAS in the environment; accordingly, this work investigated 45 legacy and emerging PFAS in samples of surface sediments and sediment cores (1940s-2020s) collected in the Pearl River outlets, its estuary, and the adjacent northern South China Sea (NSCS), one of the global pollution hotspots. The range of total PFAS concentrations in surface sediments from the river outlets and the NSCS was 244-14400 pg/g dry weight (dw) and 31.6-363 pg/g dw, respectively. In sediment cores, perfluorooctanesulfonate (PFOS) concentrations initially increased and then declined around ten years ago. Levels of long-chain perfluorinated carboxylates have been increasing since the 1980s and experienced an accelerated rise in the 2000s. Hydrogen-substituted polyfluoroalkyl ether sulfonate (H-PFESA) was widely found in sediment samples for the first time. The ratios of 6:2 H-PFESA to 6:2 chlorinated (Cl-) PFESA in sediment cores exceeded those in surface sediment and exhibited an increasing trend with the sediment age, implying the gradual transformation of 6:2 Cl-PFESA to its hydrogen-substituted analog in sediments. A preliminary risk assessment indicated that ∑6:2 PFESAs and PFOS posed medium to high risks over recent decades.

Indexed as

FluorocarbonsGeologic SedimentsAlkanesulfonic AcidsChinaEnvironmental MonitoringEstuariesRiversWater Pollutants, ChemicalAlkanesulfonic AcidsFluorocarbonsWater Pollutants, ChemicalCl-PFESAF-53BH-PFESAPFECHSsediment coretemporal trend

Identifiers

PMID40172133
PMCPMC12713727

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.