ArticleChemistry (Weinheim an der Bergstrasse, Germany)2025
Self-Sensitized Fulgimides with Selective Multiplicity-Based Three-State Photoswitching.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Precise control over excited-state multiplicity is a powerful strategy for controlling photochemical reactivity, particularly in multimodal systems where different multiplicities lead to distinct reaction products. Here, we present a multiplicity-sensitive, multimodal, fulgimide-based system capable of three-state photoswitching both in solution and in the solid state. With the aim of suppressing singlet-state sensitization, we rationally designed an intramolecularly sensitized system that enables triplet-exclusive energy transfer-a crucial feature for selective multiplicity-dependent reactivity. Our findings provide insights into the underlying principles of intramolecular triplet-exclusive sensitization and its application in controlling three-state photoswitching in unimolecular systems.
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