Evidence map›Paper›PMID 40106308›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2025

An Electrochemically-Driven Reconstruction Strategy to Realize Highly Crystalline Covalent Organic Frameworks for Enhanced Hydrogen Evolution Reaction.

Yuxin Ren, Shuang Li, Meidi Wang, Xue-Qian Wu, Ya-Pan Wu, Bojing Sun, Jun Zhao, Fangyuan Kang, Qichun Zhang, Dong-Sheng Li

Abstract read
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

  1. Review
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

10 authors.

Yuxin RenCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.
Shuang LiCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.
Meidi WangCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.
Xue-Qian WuCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.
Ya-Pan WuCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.
Bojing SunCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.
Jun ZhaoCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.
Fangyuan KangDepartment of Materials Science and Engineering, City University of Hong Kong, Tat Chee Avenue 83, Kowloon, Hong Kong SAR, 999077, P. R. China.
Qichun ZhangDepartment of Materials Science and Engineering, City University of Hong Kong, Tat Chee Avenue 83, Kowloon, Hong Kong SAR, 999077, P. R. China.ORCID https://orcid.org/0000-0003-1854-8659
Dong-Sheng LiCollege of Materials and Chemical Engineering, Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials, China Three Gorges University, Yichang, Hubei, 443002, P. R. China.

Funding

City University of Hong Kong 7020089City University of Hong Kong 9380117Higher Education Institutions of Hubei Province T201904Innovation and Technology Fund ITF ITS/322/22National Natural Science Foundation of China 21971143National Natural Science Foundation of China 22209098National Natural Science Foundation of China 22371165National Natural Science Foundation of China 22401172Project of Hubei Three Gorges Laboratory SC232018Project of Hubei Three Gorges Laboratory SK213002Project of Hubei Three Gorges Laboratory Z2022078
6 · The paper itself

Abstract

Developing diverse methods to approach highly crystalline covalent organic frameworks (COFs) for improvement of their electrocatalytic hydrogen evolution reaction (HER) activity is important but very challenging. Herein, for the first time, an electrochemically-driven reconstruction strategy is demonstrated to convert semi-polymerized low-crystalline COFs into highly crystalline, structurally ordered COFs with enhanced HER activity. In situ and ex situ characterizations reveal that cyclic voltammetry (CV) cycles can promote crystallinity, thereby leading to improved conductivity, increased active site density, and superior stability. As a result, the highly crystalline COF achieves low overpotentials of 103.6 and 219.4 mV at 10 and 50 mA cm

Indexed as

covalent organic frameworkselectrochemically driven reconstructionhigh‐crystallinityhydrogen evolution reaction

Identifiers

PMID40106308
PMCPMC12079546

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.