ArticleJournal of chemical theory and computation2025
Quantitative Theory for Critical Conditions of Like-Charge Attraction between Polarizable Spheres.
Article in Journal of chemical theory and computation, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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Who cites it
1 citing paper in PubMed.
- Charge-Induced Polarization in Dielectric Particle Systems: A Geometry-Dependent Effect.Journal of chemical theory and computation · 2025Article
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Authors and funding
2 authors.
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Abstract
Despite extensive experimental and theoretical efforts, a concise quantitative theory to predict the occurrence of like-charge attraction (LCA) between polarizable spheres remains elusive. In this work, we first derive a novel three-point image formula, based on a key observation that connects the classical Neumann's image principle with the incomplete beta function. This approach naturally yields simple yet precise critical conditions for LCA, with a relative discrepancy of less than 1% compared to numerical simulations, validated across diverse parameter settings. The obtained critical conditions may provide physical insights into various processes potentially involving LCA, such as self-assembly, crystallization, and phase separation, across different length scales. Additionally, the new image formula is directly applicable to enhance the efficiency of polarizable force field calculations involving polarizable spheres.
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