ArticleNature communications2025
General synthesis of covalent organic frameworks under ambient condition within minutes via microplasma electrochemistry approach.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Beyond solvothermal synthesis: construction of covalent organic frameworks at near-ambient conditions.Science advances · 2026Article
- Electro-assisted control over zeolite crystallization and modification: theory, configuration, and applications.Journal of materials chemistry. A · 2026Review
- Breaking π-π Stacking in One-Dimensional Covalent Organic Frameworks.Angewandte Chemie (International ed. in English) · 2026Article
- Super Cost-Effective and Scalable Imine-Based Sorbent With Field Attraction and In Situ Fixation for Efficient Capture of Diverse Iodine Species under Industrial Conditions.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Potential of Covalent Organic Framework in Pharmacy and Biomedicine: Influence of Structure on Properties and Applications.ChemMedChem · 2026Review
- Article
- Automatic Blood Protein Enrichment by Magnetic-COF Polymers.Analytical chemistry · 2026Article
- In Situ Synthesis of Covalent Organic Frameworks Inside Cells for Triggering Ferroptosis and Immunotherapy.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Hidden Structural Colors from Bistable, Electrically Driven Covalent Organic Framework Photonic Assemblies for Secure Optical Encoding.ACS nano · 2026Article
Corrections and comments
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Authors and funding
8 authors.
Funding
Abstract
Covalent organic frameworks (COFs) are typically synthesized using solvothermal conditions with high temperature and long reaction time (≥120 °C, >72 h). Herein, we report a general and rapid microplasma electrochemistry strategy to synthesize COFs under ambient conditions. A series of flexible imine-bond COFs with high-crystallinity were prepared in minutes via this method, which showed 1000-fold higher space-time yield than solvothermal method. This approach also achieved the preparation of COFs with diverse linkages including rigid imine, hydrazone, β-ketoenamies and azine linkages. Moreover, four types of imine-based COFs were successfully synthesized in aqueous acetic acid, which avoided the use of harmful organic solvents, indicating that microplasma method is green and versatile for COF synthesis. The obtained COFs showed higher surface area and exhibited superior performance in volatile iodine uptake compared to those COFs prepared by solvothermal method. After screening more than ten types of COFs, the iodine adsorption capacity could be promoted from 2.81 to 6.52 g g
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.