ArticleNature communications2025
Post-modulation of layer-by-layer assemblies coordinated by a catalytic dose of fullerene derivatives without external fields.
Bi-Jun Geng, Yun-Fei Li, Lin-Long Deng, Tong-Ruo Diao, Zi-Wei Ma, Long-Xing Lin, Jin-Shu Li, Yi-Dong Yan, Jia-Wei Yan, Yuan-Zhi Tan and 4 more
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In one paragraphArticle in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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4 · The recordCorrections and comments
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5 · Who and what moneyAuthors and funding
14 authors.
Bi-Jun Geng *Pen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.
Yun-Fei Li *Pen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.ORCID http://orcid.org/0009-0001-4009-684X Lin-Long Deng *Pen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.ORCID http://orcid.org/0000-0002-8588-1825 Tong-Ruo DiaoPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.
Zi-Wei MaPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.
Long-Xing LinPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.
Jin-Shu LiPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.
Yi-Dong YanPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.ORCID http://orcid.org/0009-0004-5457-3776 Jia-Wei YanPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.ORCID http://orcid.org/0000-0002-0045-6169 Yuan-Zhi TanPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.ORCID http://orcid.org/0000-0002-1268-2761 Bing-Wei MaoPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.
Su-Yuan XiePen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.ORCID http://orcid.org/0000-0003-2370-9947 Zhong-Qun TianPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China.ORCID http://orcid.org/0000-0002-9775-8189 Yang YangPen-Tung Sah Institute of Micro-Nano Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, China. yangyang@xmu.edu.cn.ORCID http://orcid.org/0000-0003-1967-3398 Funding
National Natural Science Foundation of China (National Science Foundation of China) 21991130National Natural Science Foundation of China (National Science Foundation of China) 21991131National Natural Science Foundation of China (National Science Foundation of China) 22032004National Natural Science Foundation of China (National Science Foundation of China) T2222002
6 · The paper itselfAbstract
Molecular assembly has attracted wide attention in chemistry, condensed physics, molecular electronics, and materials sciences. However, it remains a great challenge to perform post-modulation on the assembled structures without the aid of externally applied fields. Herein, we demonstrate a combined full-weak-bonded interaction and fullerene-derivative strategy and achieve the post-modulation of layer-by-layer assembly with a precision of 5.0 Å. In the absence of external fields, the fullerene derivative exhibits a long-range interaction to boost the modulation of the assembly. Benefiting from that, a catalytic dose of fullerene derivative is able to modulate a large area of assembly, reminiscent of the catalyst in chemical reactions. This work provides an efficient and flexible approach for the catalysis and precise modulation of molecular assembly.
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PMID40055322
PMCPMC11889154
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