ArticleNature materials2025
Operando-informed precatalyst programming towards reliable high-current-density electrolysis.
Article in Nature materials, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 16 papers.
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Who cites it
16 citing papers in PubMed.
- Electrocatalysis and Photoelectrocatalysis: Perspective from Physicochemical Mechanisms to Applications.ACS omega · 2026Review
- Customized O─O Radical Coupling Route on High-Density Fe─N─C Catalysts for Stable Industrial-Scale Water Oxidation.Angewandte Chemie (International ed. in English) · 2026Article
- Ridge catalysis unlocking water oxidation activity of pentlandite.Nature communications · 2026Article
- Linking Synthetic Materials Chemistry to Electrocatalytic Performance.Angewandte Chemie (International ed. in English) · 2026Review
- Decoupling electron transfer defines a quantitative kinetic framework for oxygen evolution catalysis.Nature communications · 2026Article
- Evaluating the Effects of Anode Porous Transport Layer on the Performance and Durability of Anion Exchange Membrane Electrolyzers.ACS omega · 2026Article
- Microwave Field Enhancement at Metal-Electrolyte Interfaces Enables Rapid Growth of Fe-NiSmall science · 2026Article
- Leveraging the kinetic isotope effect by compact H-bond motifs for electrochemical hydrogen isotope separation.Proceedings of the National Academy of Sciences of the United States of America · 2026Article
- Molecular level combination of coordination and interfacial regulations via functional ligands for industrial AEM water electrolysis.Science advances · 2026Article
- Article
- Harnessing the structural evolution of metal-organic frameworks under electrocatalytic conditions.Communications chemistry · 2025Review
- High entropy alloys for advanced electrocatalysis with computational insights and multidisciplinary design strategies.iScience · 2025Review
- Coordination-tailored atomic interfaces for selective CHNature communications · 2025Article
- Accelerated Electro-Conversion of a Nickel Coordination Complex for Hybrid Water Electrolysis.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Rolling carbon on a rock.Nature materials · 2025Article
- Layers split and zip for phase transition.Nature materials · 2025Article
Corrections and comments
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Authors and funding
29 authors.
Funding
Abstract
Electrocatalysts support crucial industrial processes and emerging decarbonization technologies, but their design is hindered by structural and compositional changes during operation, especially at application-relevant current densities. Here we use operando X-ray spectroscopy and modelling to track, and eventually direct, the reconstruction of iron sulfides and oxides for the oxygen evolution reaction. We show that inappropriate activation protocols lead to uncontrollable Fe oxidation and irreversible catalyst degradation, compromising stability and reliability and precluding predictive design. Based on these, we develop activation programming strategies that, considering the thermodynamics and kinetics of surface reconstruction, offer control over precatalyst oxidation. This enables reliable predictions and the design of active and stable electrocatalysts. In a Ni
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40021826What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.