ArticleWater science and technology : a journal of the International Association on Water Pollution Research2025
Z-scheme heterojunction BiOBr/MIL-100(Fe) visible photocatalytic-permonosulfate degradation of AO7.
Article in Water science and technology : a journal of the International Association on Water Pollution Research, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Metal-organic frameworks (MOFs) have garnered significant interest in the field of photocatalysis. In this study, Z-scheme heterojunction BM-x composites consisting of bismuth bromide oxide (BiOBr) and iron-based metal-organic backbone (MIL-100(Fe)) were successfully synthesized using ethylene glycol as a solvent. The composites were characterized using various techniques. BM-x exhibit abundant functional groups, large specific surface areas, and narrow band gap energy, thus provide numerous active sites for catalytic reactions and respond well to visible light. Notably, BM-7 displays remarkable catalytic activity in a visible light-activated permonosulfate (PMS) system and achieves a degradation rate of 99.02% over 100 mg/L gold orange II (AO7) within 60 min. The effects of BM-7 and PMS addition, initial AO7 concentration, initial pH, inorganic anions, and humic acid on the degradation system were investigated. The proposed mechanism of the Z-scheme heterojunction in the BM-7 photocatalyst demonstrates effective photoelectron transfer from the BiOBr conduction band to the MIL-100(Fe) valence band, resulting in excellent catalytic activity. Radical burst experiments identified
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