ArticleACS catalysis2025
Stoichiometric Selective Carbonylation of Methane to Acetic Acid by Chemical Looping.
Article in ACS catalysis, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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9 authors.
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Abstract
The conversion of methane to valuable products is one of the main challenges of modern chemistry. Acetic acid (AcOH) is a key chemical reagent in industry, produced nowadays by the carbonylation of methanol over homogeneous Rh and Ir catalysts. Here, we propose a stepwise chemical looping approach for the highly selective stoichiometric synthesis of AcOH by carbonylation of methane with CO using single-site Pt over isolated phosphotungstic anions on a titania support (Pt-HPW-TiO
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