ArticleSmall methods2025
Tuning Self-Assembly of Hole-Selective Monolayers for Reproducible Perovskite/Silicon Tandem Solar Cells.
Article in Small methods, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Interfacial Enhancement of Self-Assembled Monolayer by Thermal Annealing and its Impact on Perovskite Solar Cells.ChemSusChem · 2026Article
- Quantum Dot Strategies Toward Performance Improvement of Perovskite Solar Cells.Nanomaterials (Basel, Switzerland) · 2026Review
- In situ coordinated HTL strategy for high-performance and scalable perovskite solar cells.Nature communications · 2025Article
- Decoding Buried Interfaces in Perovskite Solar Cells: Core Issues, Strategic Engineering, and Prospects for High-Efficiency Stable Devices.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Review
- Tuning Self-Assembly of Hole-Selective Monolayers for Reproducible Perovskite/Silicon Tandem Solar Cells.Small methods · 2025Article
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Authors and funding
11 authors.
Funding
Abstract
Self-assemble monolayers (SAMs) have become state-of-the-art hole-selective contacts for high-efficiency perovskite-based solar cells due to their easy processing, passivation capability, and low parasitic absorption. Nevertheless, for the deposition of SAMs with a monolayer thickness and a high packing density on metal oxide substrates, critical challenges persist. To overcome these, the study focuses on the impact of annealing temperature - an intrinsic yet so far unexplored process parameter - during the formation of SAMs. By performing in situ angle-resolved X-ray photoelectron spectroscopy combined with advanced data analysis routines, it is revealed that increasing the annealing temperature reduces the formed SAM layer thickness from a multilayer stack of ≈5 nm at 100 °C (conventional temperature employed in literature) to a monolayer at 150 °C. Furthermore, denser adsorption of the SAM to the metal oxide surface is promoted at high temperatures, which enhances the interfacial SAM/perovskite passivation quality. With this strategy, a 1.3%
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