Global Spectral Analysis of Polaritonic Coupling of Multiple Organic Dyes to a Tunable Fabry-Pérot Resonator Operating with Mirror Separations up to 10 μm.

Christoph Kertzscher, Michael Mauch, Jakob Keck, Alfred J Meixner

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Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

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1citing papers in PubMed

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1 citing paper in PubMed.

Global Spectral Analysis of Polaritonic Coupling of Multiple Organic Dyes to a Tunable Fabry-Pérot Resonator Operating with Mirror Separations up to 10 μm.Chemistry (Weinheim an der Bergstrasse, Germany) · 2025
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4 authors.

Christoph KertzscherInstitute of Physical and Theoretical Chemistry, University of Tübingen, Auf der Morgenstelle 18, 72076, Tübingen, Germany.ORCID https://orcid.org/0009-0007-0684-3059

Michael MauchInstitute of Physical and Theoretical Chemistry, University of Tübingen, Auf der Morgenstelle 18, 72076, Tübingen, Germany.

Jakob KeckInstitute of Physical and Theoretical Chemistry, University of Tübingen, Auf der Morgenstelle 18, 72076, Tübingen, Germany.ORCID https://orcid.org/0000-0002-6285-8243

Alfred J MeixnerInstitute of Physical and Theoretical Chemistry, University of Tübingen, Auf der Morgenstelle 18, 72076, Tübingen, Germany.ORCID https://orcid.org/0000-0002-0187-2906

Funding

Deutsche Forschungsgemeinschaft ME 1600/13-3

6 · The paper itself

Abstract

We study strong optical coupling and the formation of hybrid polaritons by a donor-acceptor pair of J-aggregated dyes separated by up to 11 μm in a tunable Fabry-Pérot resonator. Fitting a phenomenological Hamiltonian to the white light transmission spectra of different cavity-J-aggregate-configurations, for which several hundred spectra were recorded sequentially as function of cavity length, allows us to determine coupling energies as a function of the effective cavity distances. The theoretical analysis shows that certain hybrid polaritons contain contributions from both dyes, making this system a promising platform for polariton-mediated energy transfer at very large distances.

Indexed as

Donor-acceptor systemsFabry-Pérot resonatorJ-aggregatePhotophysicsPolariton

Identifiers

PMID39992262

DOI10.1002/chem.202500344

PMCPMC11979686

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