ArticleJournal of synchrotron radiation2025
Pump-probe reciprocal-space mapping using energy-resolved XFEL pink beam pulses.
Article in Journal of synchrotron radiation, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
We present a 3D reciprocal-space mapping (RSM) method using a pink self-amplified spontaneous emission (SASE) X-ray free-electron laser beam. The energy of each specific pulse in a SASE beam can be determined using the diffraction pattern of a specimen excited by pumping itself as a spectroscopic reference. A thin slab of RSM, whose thickness corresponds to the energy bandwidth of the pink beam, is successfully reconstructed using the proposed method. By rocking a sample in a few steps, we obtained a 3D RSM covering both the diffuse scattering and the Bragg rod in NiO thin films during a pump-probe X-ray diffraction measurement.
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