ArticleAdvanced materials (Deerfield Beach, Fla.)2025
Supramolecular Engineering of Vinylene-Linked Covalent Organic Framework - Ruthenium Oxide Hybrids for Highly Active Proton Exchange Membrane Water Electrolysis.
Article in Advanced materials (Deerfield Beach, Fla.), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Accelerating Proton Transfer via Tetrahydroxy-1,4-Benzoquinone Intercalation for Enhanced Oxygen Evolution Reaction.Chemistry (Weinheim an der Bergstrasse, Germany) · 2026Article
- Wet Transfer of In Situ Grown Azo-Containing Two-Dimensional Conjugated Covalent Organic Framework Films for Photoswitchable Electronic Devices.Angewandte Chemie (International ed. in English) · 2026Article
- From Metal-Centered Catalysis to Organic Orbital Programming in Photoelectrocatalysis.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Rational Design of Covalent Organic Frameworks for Oxygen Electrocatalysis: Recent Advances and Mechanistic Insights.Nano-micro letters · 2026Review
- 3D-Printable Photothermal and Temperature-Controlled Polycaprolactone Scaffolds Incorporating Gold Plasmonic Blackbodies for Bone Tissue Engineering.ACS applied materials & interfaces · 2025Article
- Supramolecular Engineering of Vinylene-Linked Covalent Organic Framework - Ruthenium Oxide Hybrids for Highly Active Proton Exchange Membrane Water Electrolysis.Advanced materials (Deerfield Beach, Fla.) · 2025Article
Corrections and comments
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Authors and funding
11 authors.
Funding
Abstract
The controlled formation of a functional adlayer at the catalyst-water interface is a highly challenging yet potentially powerful strategy to accelerate proton transfer and deprotonation for ultimately improving the performance of proton-exchange membrane water electrolysis (PEMWE). In this study, the synthesis of robust vinylene-linked covalent organic frameworks (COFs) possessing high proton conductivities is reported, which are subsequently hybridized with ruthenium dioxide yielding high-performance anodic catalysts for the acidic oxygen evolution reaction (OER). In situ spectroscopic measurements corroborated by theoretical calculations reveal that the assembled hydrogen bonds formed between COFs and adsorbed oxo-intermediates effectively orient interfacial water molecules, stabilizing the transition states for intermediate formation of OER. This determines a decrease in the energy barriers of proton transfer and deprotonation, resulting in exceptional acidic OER performance. When integrated into a PEMWE device, the system achieves a record current density of 1.0 A cm
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Registered trials
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