ArticleNature chemistry2025
A living library concept to capture the dynamics and reactivity of mixed-metal clusters for catalysis.
Article in Nature chemistry, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Homoleptic seven-coordinate Ti(0) and Zr(0) through a new stabilization mode.Chemical science · 2026Article
- Molecular Mimics of Intermetallic Phases: Selective Alkylamide-Ligand Deprotection Drives Co/Ga Cluster Formation.Angewandte Chemie (International ed. in English) · 2026Article
- Atomically Precise Clusterzymes: A Programmable Optoelectronic Platform for Neuroscience.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Review
- Cut-SOAP: A Machine Learning Descriptor for Rapid Screening of Molecular Adsorption Energetics.ACS omega · 2026Article
- Exploring Monomer-Amino Acid Interactions in Mimicking Mips for PSA Detection-Using the Novel MBASM Approach.Journal of computational chemistry · 2025Article
- Checking out metal cluster chemistry from living libraries.Nature chemistry · 2025Article
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Authors and funding
13 authors.
Funding
Abstract
The exploration of ligated metal clusters' chemical space is challenging, partly owing to an insufficiently targeted access to reactive clusters. Now, dynamic mixtures of clusters, defined as living libraries, are obtained through organometallic precursor chemistry. The libraries are populated with interrelated clusters, including transient and highly reactive ones, as well as more accessible but less reactive species. Their evolutions upon perturbation with substrate molecules are monitored and chemical information is gained without separation of the clusters. Here we prepared a library of all-hydrocarbon ligated Cu/Zn clusters and developed a bias-free computational framework suited to analyse the full compositional space that yields a reliable structural model for each cluster. This methodology enables efficient searches for structure-reactivity relationships relevant for catalysis with mixed-metal clusters: when treating the library with CO
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Registered trials
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