ArticleScience advances2025
Advancing efficiency in deep-blue OLEDs: Exploring a machine learning-driven multiresonance TADF molecular design.
Article in Science advances, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Molecular-topology-guided multiple-resonance emitters with sub-10-nm bandwidths: ultranarrow high-efficiency solution-processable OLEDs.National science review · 2026Article
- Biomass-based thermally tunable dual afterglow with room temperature daylight visibility.Nature communications · 2026Article
- Noncovalent through-space charge transfer enables efficient and stable blue electroluminescence.Science advances · 2026Article
- Unveiling key descriptorsChemical science · 2026Article
- Complementarity fusion of boron-oxygen and carbazole blocks enables narrowband blue OLEDs with high performance.Nature communications · 2025Article
- Machine Learning-Driven Design of Fluorescent Materials: Principles, Methodologies, and Future Directions.Nanomaterials (Basel, Switzerland) · 2025Review
- Comprehensive Review on the Structural Diversity and Versatility of Multi-Resonance Fluorescence Emitters: Advance, Challenges, and Prospects toward OLEDs.Chemical reviews · 2025Review
Corrections and comments
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Authors and funding
7 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The pursuit of boron-based organic compounds with multiresonance (MR)-induced thermally activated delayed fluorescence (TADF) is propelled by their potential as narrowband blue emitters for wide-gamut displays. Although boron-doped polycyclic aromatic hydrocarbons in MR compounds share common structural features, their molecular design traditionally involves iterative approaches with repeated attempts until success. To address this, we implemented machine learning algorithms to establish quantitative structure-property relationship models, predicting key optoelectronic characteristics, such as full width at half maximum (FWHM) and main peak wavelength, for deep-blue MR candidates. Using these methodologies, we crafted ν-DABNA-O-xy and developed deep-blue organic light-emitting diodes featuring a Commission Internationale de l'Eclairage y of 0.07 and an FWHM of 19 nm. The maximum external quantum efficiency reached ca. 27.5% with a binary emission layer, which increased to 41.3% with the hyperfluorescent architecture, effectively mitigating efficiency roll-off. These findings are expected to guide the systematic design of MR-type TADF clusters, unlocking their full potential.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.