ArticleNature communications2025
Pressure treatment enables white-light emission in Zn-IPA MOF via asymmetrical metal-ligand chelate coordination.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
What it found
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The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
5 citing papers in PubMed.
- Pressure-Activated and Retained Blue Emission in Melamine Through Hydrogen-Bond and Packing Regulation.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Metal-Organic Frameworks as Programable Platforms for Micro- and Optoelectronics: From Dielectrics to Semiconductors and White-Light Emitters.Small science · 2026Article
- Pressure-driven steric hindrance engineering for maximizing photoluminescence in covalent organic frameworks.Science advances · 2026Article
- Coordination-Locked Engineering to Achieve Narrowband Room Temperature Phosphorescence in Non-Rare Earth Metal-Organic Frameworks.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Pressure-Modulated Host-Guest Interactions Boost Effective Blue-Light Emission of MIL-140A Nanocrystals.Nano-micro letters · 2025Article
Corrections and comments
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Authors and funding
7 authors.
Funding
Abstract
Metal-organic frameworks that feature hybrid fluorescence and phosphorescence offer unique advantages in white-emitting communities based on their multiple emission centers and high exciton utilization. However, it poses a substantial challenge to realize superior white-light emission in single-component metal-organic frameworks without encapsulating varying chromophores or integrating multiple phosphor subunits. Here, we achieve a high-performance white-light emission with photoluminescence quantum yield of 81.3% via boosting triplet excitons distribution through pressure treatment in single-component Zn-IPA metal-organic frameworks. A novel metal-ligand asymmetrical chelate coordination is successfully integrated into the Zn-IPA after a high-pressure treatment over ~20.0 GPa. This modification unexpectedly endows the targeted sample with a new emergent electronic state to narrow the singlet-triplet energy gap, which effectively accelerates the spin-flipping process for boosted triplet excitons population. Time delay phosphor-converted light-emitting diodes are fabricated with long emission time up to ~7 s after switching off, providing significant advancements for white-light and time-delay lighting applications.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.