ArticleScience advances2025
Soft nanoforest of metal single atoms for free diffusion catalysis.
Article in Science advances, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Halogen Bonding-Sustained Accumulation of Polyiodide in Hierarchically Open Micellar Film for Shuttle-Free Long-Duration Zn-IAngewandte Chemie (International ed. in English) · 2026Article
- Asymmetric Ru─O sites in self-activated catalysts for efficient electrochemical methanol oxidation and industrial-scale hydrogen generation.Science advances · 2026Article
- Self-Disproportionation-Induced H-Adsorption/Desorption Zones in Amorphous Nickel Boride Cocatalyst for Efficient Photocatalytic Hydrogen Evolution.Journal of the American Chemical Society · 2026Article
- Programmable Interface Atomic Rearrangement for Spatiotemporal Thermal Radiation Tailoring.Research (Washington, D.C.) · 2026Article
- Bioinspired Design of Heterogenous Single-Atomic-Site Catalysts for Electrocatalysis and Photocatalysis.Advanced materials (Deerfield Beach, Fla.) · 2025Review
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Authors and funding
11 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Metal single atoms are of increasing importance in catalytic reactions. However, the mass diffusion is yet substantially limited by the confined surface of the support in comparison to homogeneous catalysis. Here, we demonstrate that cylindrical micellar brushes with highly solvated poly(2-vinylpyridine) coronas can immobilize 33 types of metal single atoms with 8.3 to 40.9 weight % contents on conventional electrodes under ambient conditions. This is favored by the forest-like hierarchically open soft structure of the micellar brushes and the dynamic coordination between the metals and the pyridine groups. It was found that the nanoforests of individual noble metal single atoms can be well solvated in an aqueous electrolyte to comprehensively expose the atomic active sites and the nanoforest of Pt single atoms on nickel foam reveals high electrochemical performance for hydrogen evolution. The micellar brush support also enables the simultaneous anchoring of multiple single atoms on the cathode of an anion-exchange membrane electrolyzer for long-term stable water electrolysis.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.