ArticleACS nano2025
Individual Assembly of Radical Molecules on Superconductors: Demonstrating Quantum Spin Behavior and Bistable Charge Rearrangement.
Article in ACS nano, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
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Who cites it
11 citing papers in PubMed.
- Non-equilibrium correlated electron dynamics in triangular molecular assemblies.Nature communications · 2026Article
- Scanning Tunnelling Microscopy Study of Spin Interactions in Transition-Metal Phthalocyanine Adsorbates: Mechanisms, Signatures, and Control Strategies.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Review
- First Access to Tetraazadiindenopyrenes via Selective Pyrrole Cyclization of Phenyl-Substituted Tetraazapyrene Derivatives on Au(111).Small science · 2026Article
- Magnetic properties of molecules on surfaces studied with scanning probe methods.National science review · 2026Review
- Locally induced Stark shifts of collective excitonic modes in polyradical aggregates.Beilstein journal of nanotechnology · 2026Article
- Connectivity Effect on Electronic Properties of Azulene-Tetraazapyrene Triads.Molecules (Basel, Switzerland) · 2025Article
- Toward Gate-Tunable Topological Superconductivity in a Supramolecular Electron Spin Lattice.Nano letters · 2025Article
- Cascade C-H Halogenation of Tetraazapyrene with Iodine Halides.Organic letters · 2025Article
- Discharge and electron correlation of radical molecules in a supramolecular assembly on superconducting Pb(111).Nanoscale horizons · 2025Article
- Probing Molecular Properties at Atomic Length Scale Using Charge-State Control.Chemical reviews · 2025Review
- Adsorption-Site- and Orientation-Dependent Magnetism of a Molecular Switch on Pb(100).ACS nano · 2025Article
Corrections and comments
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Authors and funding
12 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
High-precision molecular manipulation techniques are used to control the distance between radical molecules on superconductors. Our results show that the molecules can host single electrons with a spin 1/2. By changing the distance between tip and sample, a quantum phase transition from the singlet to doublet ground state can be induced. Due to local screening and charge redistribution, we observe either charged or neutral molecules, which couple in a sophisticated way, showing quantum spin behavior that deviates from the classical spins. Dimers at different separations show multiple Yu-Shiba-Rusinov peaks in tunneling spectroscopy of varying intensity, which are in line with the superconducting two-impurity Anderson model, where singlet (
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.