ArticleNature materials2025
Resolving and routing magnetic polymorphs in a 2D layered antiferromagnet.
Article in Nature materials, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
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Who cites it
13 citing papers in PubMed.
- Layer photovoltaic effect in a two-dimensional antiferromagnet with parity-time symmetry.Nature materials · 2026Article
- Hybrid Superconducting-Magnetic Van der Waals Heterostructures: Physics and Application.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Layer-number-parity-dependent abnormal magnetic ordering in few-layer CrI3 on N-face AlN substrate.Nature communications · 2026Article
- Magneto-optical Kerr effect in an A-type antiferromagnet.Nature communications · 2026Article
- Article
- Terahertz Electronic and Spin Currents in Wafer-Scale Van der Waals BiAdvanced materials (Deerfield Beach, Fla.) · 2026Article
- Doping-induced magnetic phase transition enables all-electrical spin control in CrSBr.Nature communications · 2025Article
- Lateral exchange bias for Néel-vector control in atomically thin antiferromagnets.Nature communications · 2025Article
- Charge transfer governed interlayer magnetic coupling and symmetry breaking in a van der Waals magnet.Nature communications · 2025Article
- Configurable antiferromagnetic domains and lateral exchange bias in atomically thin CrPSNature materials · 2025Article
- Roadmap for Photonics with 2D Materials.ACS photonics · 2025Review
- Spin-chirality-driven second-harmonic generation in two-dimensional magnet CrSBr.Science advances · 2025Article
- A Polycarbonate-Assisted Transfer Method for van der Waals Contacts to Magnetic Two-Dimensional Materials.Micromachines · 2024Article
Corrections and comments
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Authors and funding
14 authors.
Funding
Abstract
Polymorphism, commonly denoting diverse molecular or crystal structures, is crucial in the natural sciences. In van der Waals antiferromagnets, a new type of magnetic polymorphism arises, presenting multiple layer-selective magnetic structures with identical total magnetization. However, resolving and manipulating such magnetic polymorphs remain challenging. Here, phase-resolved magnetic second harmonic generation microscopy is used to elucidate magnetic polymorphism in 2D layered antiferromagnet CrSBr, demonstrating deterministic and layer-selective switching of magnetic polymorphs. Using a nonlinear magneto-optical technique, we unambiguously resolve the polymorphic spin-flip transitions in CrSBr bilayers and tetralayers through both the amplitude and phase of light. Remarkably, the deterministic routing of polymorphic spin-flip transitions originates from a 'layer-sharing' effect, where the transitions are governed by laterally extended layers acting as 'control bits'. We envision that such controllable magnetic polymorphism could be ubiquitous for van der Waals layered antiferromagnets, enabling new designs and constructions of spintronic and opto-spintronic devices for probabilistic computation and neuromorphic engineering.
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Registered trials
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