ArticlePolymers2025
In Situ Raman Spectroscopy-Enabled Microfluidic Gel Chromatography for Revealing Real-Time Separation Dynamics of Single-Walled Carbon Nanotubes.
Article in Polymers, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Single-walled carbon nanotubes (SWNTs) exhibit distinct electronic properties, categorized as metallic or semiconducting, determined by their chirality. The precise and selective separation of these electronic types is pivotal for advancing nanotechnology applications. While conventional gel chromatography has been widely employed for large-scale separations, its limitations in addressing microscale dynamics and electronic-type differentiation have persisted. Here, we present a polydimethylsiloxane (PDMS)-based microfluidic gel chromatography platform, coupled with real-time in situ Raman spectroscopy, designed to achieve the high-resolution electronic-type separation of SWNTs. This platform systematically isolates metallic- and semiconducting-enriched fractions (M1-M3 and S1-S3) while quantitatively analyzing separation dynamics through G-band spectral shifts and G
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