ArticleACS materials letters2025
Probing the Design Rules for Optimizing Electron Spin Relaxation in Densely Packed Triplet Media for Quantum Applications.
Article in ACS materials letters, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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Who cites it
1 citing paper in PubMed.
- Chemically Tuning Room Temperature Pulsed Optically Detected Magnetic Resonance.Journal of the American Chemical Society · 2025Article
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Authors and funding
8 authors.
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Abstract
Quantum technologies using electron spins have the advantage of employing chemical qubit media with tunable properties. The principal objective of material engineers is to enhance photoexcited spin yields and quantum spin relaxation. In this study, we demonstrate a facile synthetic approach to control spin properties in charge-transfer cocrystals consisting of 1,2,4,5-tetracyanobenzene (TCNB) and acetylated anthracene. We find that the extent and position of acetylation control the degree of charge-transfer and the optical band gap by modifying crystal packing and electronic structure. We further reveal that while the spin polarization of the triplet state is slightly reduced compared to prototypical Anthracene:TCNB, the phase memory (
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